JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, cilt.251, sa.3, ss.251-259, 2002 (SCI-Expanded)
The various magnetic structures of the ThCr2Si2 structured RMn2Ge2 (R: rare-earth) compounds can lead to numerous magnetic configurations by gradually substituting the rare-earth element by another lanthanide. In this study, the magnetic properties of Nd1-xDyxMn2Ge2 (0 less than or equal to x less than or equal to 1) compounds were investigated by means of temperature-dependent DC magnetization measurements in low external magnetic fields. The substitution of Dy for Nd leads to a linear decrease in the lattice constants, and the magnetic interactions in the Mn sublattice cross over from a ferromagnetic character to an antiferromagnetic one. At low temperatures, the rare-earth sublattice orders in various configurations that depend on the composition. The results are collected in a phase diagram. (C) 2002 Elsevier Science B.V. All rights reserved.