Thermal stability of the Merck quartz CW-OSL and EPR signals


KAYA KELEŞ Ş., POLYMERIS G., MERİÇ N.

Sixth International Conference on Radiation and Applications in Various Fields of Research (RAD 2018), Ohrid, Makedonya, 18 - 22 Haziran 2018

  • Yayın Türü: Bildiri / Özet Bildiri
  • Basıldığı Şehir: Ohrid
  • Basıldığı Ülke: Makedonya
  • Ankara Üniversitesi Adresli: Evet

Özet

Quartz is the most common mineral in luminescence dating and retrospective dosimetry studies

for reconstruction of either radiation dose in an accident or equivalent dose of archaeological materials.

For dose assessment, luminescence intensity of irradiated sample is compared with the intensity of the

sample irradiated with known dose in the laboratory. The intensity can be obtained by the method

based on optically stimulating called Optically Stimulated Luminescence (OSL). Also Electron

Paramagnetic Resonance (EPR) is a technique based on the detection of paramagnetic defects that are

proportional to the absorbed radiation dose within the material. Thermal stability is one of the

essential properties for a material to be useful in dosimetry studies. Trap centers must be enough stable

to accumulate the radiation dose until the time of measurement. For irradiation, heating and

monitoring the CW-OSL signals, Risø TLDA 20 reader which has an internal 90Sr/90Y beta source was

used. Luminescence emission was detected through U-340 filter. Merck quartz samples were

irradiated with 300 Gy for both CW-OSL and EPR measurements. For thermal stability, samples were

heated from room temperature (~20°C) up to 425°C by the steps of 25°C with a heating rate of 1°C/s,

after monitoring the blue stimulated OSL signals, EPR measurements were done. EPR measurements

were carried out using X-band (∼10 GHz) using a Bruker EMX spectrometer In this study, thermal

stability of Merck quartz CW-OSL and EPR signals were investigated and we tried to see whether there

is a correlation between these two signals. As a result, CW-OSL and EPR signal intensities are similar

with heating between room temperature and 425°C. Both signals were stable up to 250 °C and started

to decrease after this temperature. Above 375°C the signals are totally depleted. By considering the

thermal stability behaviour of CW-OSL and EPR signals, we may talk about a possible correlation

between them.